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	<journal>
		<journal_title>Biogeosciences</journal_title>
		<journal_url>www.biogeosciences.net</journal_url>
		<issn>1726-4170</issn>
		<eissn>1726-4189</eissn>
		<volume_number>6</volume_number>
		<issue_number>12</issue_number>
		<publication_year>2009</publication_year>
	</journal>
	<doi>10.5194/bg-6-2847-2009</doi>
	<article_url>http://www.biogeosciences.net/6/2847/2009/</article_url>
	<abstract_html>http://www.biogeosciences.net/6/2847/2009/bg-6-2847-2009.html</abstract_html>
	<fulltext_pdf>http://www.biogeosciences.net/6/2847/2009/bg-6-2847-2009.pdf</fulltext_pdf>
	<start_page>2847</start_page>
	<end_page>2860</end_page>
	<publication_date>2009-12-04</publication_date>
	<article_title content_type="html">Estimation of NH&lt;sub&gt;3&lt;/sub&gt; emissions from a naturally ventilated livestock farm using local-scale atmospheric dispersion modelling</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>A. Hensen</name>
			<email>hensen@ecn.nl</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>B. Loubet</name>
		</author>
		<author numeration="3" affiliations="1,6">
			<name>J. Mosquera</name>
		</author>
		<author numeration="4" affiliations="1">
			<name>W. C. M. van den Bulk</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>J. W. Erisman</name>
		</author>
		<author numeration="6" affiliations="3">
			<name>U. DÃ¤mmgen</name>
		</author>
		<author numeration="7" affiliations="4">
			<name>C. Milford</name>
		</author>
		<author numeration="8" affiliations="3">
			<name>F. J. LÃ¶pmeier</name>
		</author>
		<author numeration="9" affiliations="2">
			<name>P. Cellier</name>
		</author>
		<author numeration="10" affiliations="5">
			<name>P. MikuÅ¡ka</name>
		</author>
		<author numeration="11" affiliations="4">
			<name>M. A. Sutton</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Energy research Centre of the Netherlands (ECN), Petten, The Netherlands</affiliation>
		<affiliation numeration="2" content_type="html">Institut National de la Recherche Agronomique (INRA), Thiverval-Grignon, France</affiliation>
		<affiliation numeration="3" content_type="html">Federal Agricultural Research Centre, Braunschweig (FAL), Germany</affiliation>
		<affiliation numeration="4" content_type="html">Centre for Ecology and Hydrology (CEH), Edinburgh, UK</affiliation>
		<affiliation numeration="5" content_type="html">Institute of Analytical Chemistry, ASCR, v.v.i., Brno, Czech Republic</affiliation>
		<affiliation numeration="6" content_type="html">now at: Animal Sciences Group (ASG), Wageningen, Germany</affiliation>
	</affiliations>
	<abstract content_type="html">Agricultural livestock represents the main source of ammonia (NH&lt;sub&gt;3&lt;/sub&gt;) in
Europe. In recent years, reduction policies have been applied to reduce
NH&lt;sub&gt;3&lt;/sub&gt; emissions. In order to estimate the impacts of these policies,
robust estimates of the emissions from the main sources, i.e. livestock
farms are needed. In this paper, the NH&lt;sub&gt;3&lt;/sub&gt; emissions were estimated from
a naturally ventilated livestock farm in Braunschweig, Germany during a
joint field experiment of the GRAMINAE European project. An inference method
was used with a Gaussian-3D plume model and with the Huang 3-D model.
NH&lt;sub&gt;3&lt;/sub&gt; concentrations downwind of the source were used together with
micrometeorological data to estimate the source strength over time. Mobile
NH&lt;sub&gt;3&lt;/sub&gt; concentration measurements provided information on the spatial
distribution of source strength. The estimated emission strength ranged
between 6.4&amp;plusmn;0.18 kg NH&lt;sub&gt;3&lt;/sub&gt; d&lt;sup&gt;&amp;minus;1&lt;/sup&gt; (Huang 3-D model) and 9.2&amp;plusmn;0.7 kg
NH&lt;sub&gt;3&lt;/sub&gt; d&lt;sup&gt;&amp;minus;1&lt;/sup&gt; (Gaussian-3D model). These estimates were 94%
and 63% of what was obtained using emission factors from the German
national inventory (9.6 kg d&lt;sup&gt;&amp;minus;1&lt;/sup&gt; NH&lt;sub&gt;3&lt;/sub&gt;). The effect of deposition was
evaluated with the FIDES-2D model. This increased the emission estimate to
11.7 kg NH&lt;sub&gt;3&lt;/sub&gt; d&lt;sup&gt;&amp;minus;1&lt;/sup&gt;, showing that deposition can explain the observed
difference. The daily pattern of the source was correlated with net
radiation and with the temperature inside the animal houses. The daily
pattern resulted from a combination of a temperature effect on the source
concentration together with an effect of variations in free and forced
convection of the building ventilation rate. Further development of the
plume technique is especially relevant for naturally ventilated farms, since
the variable ventilation rate makes other emission measurements difficult.</abstract>
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